TY - JOUR
T1 - Phonon-exciton Interactions in WSe2 under a quantizing magnetic field
AU - Li, Zhipeng
AU - Wang, Tianmeng
AU - Miao, Shengnan
AU - Li, Yunmei
AU - Lu, Zhenguang
AU - Jin, Chenhao
AU - Lian, Zhen
AU - Meng, Yuze
AU - Blei, Mark
AU - Taniguchi, Takashi
AU - Watanabe, Kenji
AU - Tongay, Sefaattin
AU - Yao, Wang
AU - Smirnov, Dmitry
AU - Zhang, Chuanwei
AU - Shi, Su Fei
N1 - Funding Information:
This work is primarily supported by AFOSR through Grant FA9550-18-1-0312. T.W. and S.-F.S. acknowledge support from ACS PRF through Grant 59957-DNI10. Z. Lian and S.-F.S. acknowledge support from NYSTAR through Focus Center-NY–RPI Contract C150117. The device fabrication was supported by the Micro and Nanofabrication Clean Room (MNCR) at Rensselaer Polytechnic Institute (RPI). S.T. acknowledges support from NSF DMR-1904716, DMR-1838443, and CMMI-1933214. K.W. and T.T. acknowledge support from the Elemental Strategy Initiative conducted by the MEXT, Japan and the CREST (JPMJCR15F3), JST. Z. Lu and D.S. acknowledge support from the US Department of Energy (DE-FG02-07ER46451) for magneto-photoluminescence measurements performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation through NSF/DMR-1644779 and the State of Florida. Y.L. and C.Z. are supported by AFOSR (Grant No. FA9550-16-1-0387), NSF (Grant No. PHY-1806227), and ARO (Grant No. W911NF-17-1-0128). S.-F.S. also acknowledges the support from NSF through Grant DMR-1945420, the support from a KIP grant from RPI, and a VSP grant from NHMFL.
Publisher Copyright:
© 2020, The Author(s).
PY - 2020/12/1
Y1 - 2020/12/1
N2 - Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to modify the exciton-phonon interactions by quantizing excitons into discrete Landau levels, which is largely unexplored. Here, we observe the Landau levels originating from phonon-exciton complexes and directly probe exciton-phonon interaction under a quantizing magnetic field. Phonon-exciton interaction lifts the inter-Landau-level transition selection rules for dark trions, manifested by a distinctively different Landau fan pattern compared to bright trions. This allows us to experimentally extract the effective mass of both holes and electrons. The onset of Landau quantization coincides with a significant increase of the valley-Zeeman shift, suggesting strong many-body effects on the phonon-exciton interaction. Our work demonstrates monolayer WSe2 as an intriguing playground to study phonon-exciton interactions and their interplay with charge, spin, and valley.
AB - Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to modify the exciton-phonon interactions by quantizing excitons into discrete Landau levels, which is largely unexplored. Here, we observe the Landau levels originating from phonon-exciton complexes and directly probe exciton-phonon interaction under a quantizing magnetic field. Phonon-exciton interaction lifts the inter-Landau-level transition selection rules for dark trions, manifested by a distinctively different Landau fan pattern compared to bright trions. This allows us to experimentally extract the effective mass of both holes and electrons. The onset of Landau quantization coincides with a significant increase of the valley-Zeeman shift, suggesting strong many-body effects on the phonon-exciton interaction. Our work demonstrates monolayer WSe2 as an intriguing playground to study phonon-exciton interactions and their interplay with charge, spin, and valley.
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U2 - 10.1038/s41467-020-16934-x
DO - 10.1038/s41467-020-16934-x
M3 - Article
C2 - 32561746
AN - SCOPUS:85086639021
SN - 2041-1723
VL - 11
JO - Nature communications
JF - Nature communications
IS - 1
M1 - 3104
ER -