Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Rebecca Boll; Arnaud Rouzée; Marcus Adolph; Denis Anielski; Andrew Aquila; Sadia Bari; Cédric Bomme; Christoph Bostedt; John D. Bozek; Henry N. Chapman; Lauge Christensen; Ryan Coffee; Niccola Coppola; Sankar De; Piero Decleva; Sascha W. Epp; Benjamin Erk; Frank Filsinger; Lutz Foucar; Tais Gorkhover; Lars Gumprecht; André Hömke; Lotte Holmegaard; Per Johnsson; Jens S. Kienitz; Thomas Kierspel; Faton Krasniqi; Kai Uwe Kühnel; Jochen Maurer; Marc Messerschmidt; Robert Moshammer; Nele L.M. Müller; Benedikt Rudek; Evgeny Savelyev; Ilme Schlichting; Carlo Schmidt; Frank Scholz; Sebastian Schorb; Joachim Schulz; Jörn Seltmann; Mauro Stener; Stephan Stern; Simone Techert; Jan Thøgersen; Sebastian Trippel; Jens Viefhaus; Marc Vrakking; Henrik Stapelfeldt; Jochen Küpper; Joachim Ullrich; Artem Rudenko; Daniel Rolles

doi:10.1039/c4fd00037d

Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Rebecca Boll, Arnaud Rouzée, Marcus Adolph, Denis Anielski, Andrew Aquila, Sadia Bari, Cédric Bomme, Christoph Bostedt, John D. Bozek, Henry N. Chapman, Lauge Christensen, Ryan Coffee, Niccola Coppola, Sankar De, Piero Decleva, Sascha W. Epp, Benjamin Erk, Frank Filsinger, Lutz Foucar, Tais GorkhoverLars Gumprecht, André Hömke, Lotte Holmegaard, Per Johnsson, Jens S. Kienitz, Thomas Kierspel, Faton Krasniqi, Kai Uwe Kühnel, Jochen Maurer, Marc Messerschmidt, Robert Moshammer, Nele L.M. Müller, Benedikt Rudek, Evgeny Savelyev, Ilme Schlichting, Carlo Schmidt, Frank Scholz, Sebastian Schorb, Joachim Schulz, Jörn Seltmann, Mauro Stener, Stephan Stern, Simone Techert, Jan Thøgersen, Sebastian Trippel, Jens Viefhaus, Marc Vrakking, Henrik Stapelfeldt, Jochen Küpper, Joachim Ullrich, Artem Rudenko, Daniel Rolles

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Abstract

This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C₈H₅F) and dissociating, laser-aligned 1,4-dibromobenzene (C₆H₄Br₂) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.

Original language	English (US)
Pages (from-to)	57-80
Number of pages	24
Journal	Faraday Discussions
Volume	171
DOIs	https://doi.org/10.1039/c4fd00037d
State	Published - Dec 1 2014
Externally published	Yes

ASJC Scopus subject areas

Medicine(all)

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10.1039/c4fd00037d

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Boll, R., Rouzée, A., Adolph, M., Anielski, D., Aquila, A., Bari, S., Bomme, C., Bostedt, C., Bozek, J. D., Chapman, H. N., Christensen, L., Coffee, R., Coppola, N., De, S., Decleva, P., Epp, S. W., Erk, B., Filsinger, F., Foucar, L., ... Rolles, D. (2014). Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules. Faraday Discussions, 171, 57-80. https://doi.org/10.1039/c4fd00037d

Boll, R, Rouzée, A, Adolph, M, Anielski, D, Aquila, A, Bari, S, Bomme, C, Bostedt, C, Bozek, JD, Chapman, HN, Christensen, L, Coffee, R, Coppola, N, De, S, Decleva, P, Epp, SW, Erk, B, Filsinger, F, Foucar, L, Gorkhover, T, Gumprecht, L, Hömke, A, Holmegaard, L, Johnsson, P, Kienitz, JS, Kierspel, T, Krasniqi, F, Kühnel, KU, Maurer, J, Messerschmidt, M, Moshammer, R, Müller, NLM, Rudek, B, Savelyev, E, Schlichting, I, Schmidt, C, Scholz, F, Schorb, S, Schulz, J, Seltmann, J, Stener, M, Stern, S, Techert, S, Thøgersen, J, Trippel, S, Viefhaus, J, Vrakking, M, Stapelfeldt, H, Küpper, J, Ullrich, J, Rudenko, A & Rolles, D 2014, 'Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules', Faraday Discussions, vol. 171, pp. 57-80. https://doi.org/10.1039/c4fd00037d

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title = "Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules",

abstract = "This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.",

author = "Rebecca Boll and Arnaud Rouz{\'e}e and Marcus Adolph and Denis Anielski and Andrew Aquila and Sadia Bari and C{\'e}dric Bomme and Christoph Bostedt and Bozek, {John D.} and Chapman, {Henry N.} and Lauge Christensen and Ryan Coffee and Niccola Coppola and Sankar De and Piero Decleva and Epp, {Sascha W.} and Benjamin Erk and Frank Filsinger and Lutz Foucar and Tais Gorkhover and Lars Gumprecht and Andr{\'e} H{\"o}mke and Lotte Holmegaard and Per Johnsson and Kienitz, {Jens S.} and Thomas Kierspel and Faton Krasniqi and K{\"u}hnel, {Kai Uwe} and Jochen Maurer and Marc Messerschmidt and Robert Moshammer and M{\"u}ller, {Nele L.M.} and Benedikt Rudek and Evgeny Savelyev and Ilme Schlichting and Carlo Schmidt and Frank Scholz and Sebastian Schorb and Joachim Schulz and J{\"o}rn Seltmann and Mauro Stener and Stephan Stern and Simone Techert and Jan Th{\o}gersen and Sebastian Trippel and Jens Viefhaus and Marc Vrakking and Henrik Stapelfeldt and Jochen K{\"u}pper and Joachim Ullrich and Artem Rudenko and Daniel Rolles",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry 2014.",

year = "2014",

month = dec,

day = "1",

doi = "10.1039/c4fd00037d",

language = "English (US)",

volume = "171",

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T1 - Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

AU - Boll, Rebecca

AU - Rouzée, Arnaud

AU - Adolph, Marcus

AU - Anielski, Denis

AU - Aquila, Andrew

AU - Bari, Sadia

AU - Bomme, Cédric

AU - Bostedt, Christoph

AU - Bozek, John D.

AU - Chapman, Henry N.

AU - Christensen, Lauge

AU - Coffee, Ryan

AU - Coppola, Niccola

AU - De, Sankar

AU - Decleva, Piero

AU - Epp, Sascha W.

AU - Erk, Benjamin

AU - Filsinger, Frank

AU - Foucar, Lutz

AU - Gorkhover, Tais

AU - Gumprecht, Lars

AU - Hömke, André

AU - Holmegaard, Lotte

AU - Johnsson, Per

AU - Kienitz, Jens S.

AU - Kierspel, Thomas

AU - Krasniqi, Faton

AU - Kühnel, Kai Uwe

AU - Maurer, Jochen

AU - Messerschmidt, Marc

AU - Moshammer, Robert

AU - Müller, Nele L.M.

AU - Rudek, Benedikt

AU - Savelyev, Evgeny

AU - Schlichting, Ilme

AU - Schmidt, Carlo

AU - Scholz, Frank

AU - Schorb, Sebastian

AU - Schulz, Joachim

AU - Seltmann, Jörn

AU - Stener, Mauro

AU - Stern, Stephan

AU - Techert, Simone

AU - Thøgersen, Jan

AU - Trippel, Sebastian

AU - Viefhaus, Jens

AU - Vrakking, Marc

AU - Stapelfeldt, Henrik

AU - Küpper, Jochen

AU - Ullrich, Joachim

AU - Rudenko, Artem

AU - Rolles, Daniel

PY - 2014/12/1

Y1 - 2014/12/1

N2 - This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.

AB - This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.

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DO - 10.1039/c4fd00037d

M3 - Article

AN - SCOPUS:84912008401

SN - 1359-6640

VL - 171

SP - 57

EP - 80

JO - Faraday Discussions

JF - Faraday Discussions

ER -

Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

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