Direct Measurement of Anharmonic Decay Channels of a Coherent Phonon

Samuel W. Teitelbaum, Thomas Henighan, Yijing Huang, Hanzhe Liu, Mason P. Jiang, Diling Zhu, Matthieu Chollet, Takahiro Sato, Éamonn D. Murray, Stephen Fahy, Shane O'Mahony, Trevor P. Bailey, Ctirad Uher, Mariano Trigo, David A. Reis

Research output: Contribution to journalArticlepeer-review

22 Scopus citations


We report channel-resolved measurements of the anharmonic coupling of the coherent A1g phonon in photoexcited bismuth to pairs of high wave vector acoustic phonons. The decay of a coherent phonon can be understood as a parametric resonance process whereby the atomic displacement periodically modulates the frequency of a broad continuum of modes. This coupling drives temporal oscillations in the phonon mean-square displacements at the A1g frequency that are observed across the Brillouin zone by femtosecond x-ray diffuse scattering. We extract anharmonic coupling constants between the A1g and several representative decay channels that are within an order of magnitude of density functional perturbation theory calculations.

Original languageEnglish (US)
Article number125901
JournalPhysical Review Letters
Issue number12
StatePublished - Sep 20 2018
Externally publishedYes

ASJC Scopus subject areas

  • Physics and Astronomy(all)


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