Time-resolved fluorescence of polarizable chromophores

Research output: Contribution to journalArticlepeer-review

22 Scopus citations


The fundamental problem of how a nonlinear coupling of the solute to the solvent affects time-resolved spectral line shapes and observable spectral moments is addressed. In particular, an exact solution for the time-dependent time-resolved fluorescence (TRF) line shape is given. This solution allows to analyze approximations commonly adopted in the theoretical analysis of transient spectra.

Original languageEnglish (US)
Pages (from-to)8933-8941
Number of pages9
JournalJournal of Chemical Physics
Issue number19
StatePublished - Nov 15 2001

ASJC Scopus subject areas

  • General Physics and Astronomy
  • Physical and Theoretical Chemistry


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