Single-atom catalysis in mesoporous photovoltaics: The principle of utility maximization

Yantao Shi; Chunyu Zhao; Haisheng Wei; Jiahao Guo; Suxia Liang; Aiqin Wang; Tao Zhang; Jingyue Liu; Tingli Ma

doi:10.1002/adma.201402978

Single-atom catalysis in mesoporous photovoltaics: The principle of utility maximization

Yantao Shi
, Chunyu Zhao
, Haisheng Wei
, Jiahao Guo
, Suxia Liang
, Aiqin Wang
, Tao Zhang
, Jingyue Liu
, Tingli Ma

Physics

Research output: Contribution to journal › Article › peer-review

134 Scopus citations

Abstract

(Graph Presented) FeO_x-supported single Pt atoms are used for the first time as counter electrodes (CEs) in dye-sensitized solar cells (DSCs), which are mesoporous photovoltaic devices. This system enables the investigation of the electrocatalytic behavior of a single-atom catalyst (SAC). Compared with conventional Pt CEs, the SAC-based CEs exhibit better reversibility as indicated by the peak-to-peak separation (E_pp). A high degree of atom utilization is demonstrated.

Original language	English (US)
Pages (from-to)	8147-8153
Number of pages	7
Journal	Advanced Materials
Volume	26
Issue number	48
DOIs	https://doi.org/10.1002/adma.201402978
State	Published - Oct 13 2014

Keywords

Dye-sensitized solar cells
Electrode materials
Iron oxide
Photovoltaic materials
Platinum
Single-atom catalysts

ASJC Scopus subject areas

General Materials Science
Mechanics of Materials
Mechanical Engineering

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10.1002/adma.201402978

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title = "Single-atom catalysis in mesoporous photovoltaics: The principle of utility maximization",

abstract = "(Graph Presented) FeOx-supported single Pt atoms are used for the first time as counter electrodes (CEs) in dye-sensitized solar cells (DSCs), which are mesoporous photovoltaic devices. This system enables the investigation of the electrocatalytic behavior of a single-atom catalyst (SAC). Compared with conventional Pt CEs, the SAC-based CEs exhibit better reversibility as indicated by the peak-to-peak separation (Epp). A high degree of atom utilization is demonstrated.",

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T1 - Single-atom catalysis in mesoporous photovoltaics

T2 - The principle of utility maximization

AU - Shi, Yantao

AU - Zhao, Chunyu

AU - Wei, Haisheng

AU - Guo, Jiahao

AU - Liang, Suxia

AU - Wang, Aiqin

AU - Zhang, Tao

AU - Liu, Jingyue

AU - Ma, Tingli

PY - 2014/10/13

Y1 - 2014/10/13

N2 - (Graph Presented) FeOx-supported single Pt atoms are used for the first time as counter electrodes (CEs) in dye-sensitized solar cells (DSCs), which are mesoporous photovoltaic devices. This system enables the investigation of the electrocatalytic behavior of a single-atom catalyst (SAC). Compared with conventional Pt CEs, the SAC-based CEs exhibit better reversibility as indicated by the peak-to-peak separation (Epp). A high degree of atom utilization is demonstrated.

AB - (Graph Presented) FeOx-supported single Pt atoms are used for the first time as counter electrodes (CEs) in dye-sensitized solar cells (DSCs), which are mesoporous photovoltaic devices. This system enables the investigation of the electrocatalytic behavior of a single-atom catalyst (SAC). Compared with conventional Pt CEs, the SAC-based CEs exhibit better reversibility as indicated by the peak-to-peak separation (Epp). A high degree of atom utilization is demonstrated.

KW - Dye-sensitized solar cells

KW - Electrode materials

KW - Iron oxide

KW - Photovoltaic materials

KW - Platinum

KW - Single-atom catalysts

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DO - 10.1002/adma.201402978

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SN - 0935-9648

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EP - 8153

JO - Advanced Materials

JF - Advanced Materials

IS - 48

ER -

Single-atom catalysis in mesoporous photovoltaics: The principle of utility maximization

Abstract

Keywords

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